Published July 11, 2025 | Version Published
Journal Article Open

Getting out of a tight spot: Cooperative unclogging of hydrogel particles in disordered porous media

  • 1. ROR icon Princeton University
  • 2. ROR icon University of Paris-Saclay
  • 3. ROR icon University of Pennsylvania
  • 4. ROR icon California Institute of Technology

Abstract

We use event-driven pore network modeling to study the transport of hydrogel particles through disordered porous media—a process that underlies diverse applications. By simulating particle advection, deformation, and clogging at the pore scale, we identify a dimensionless "squeezing parameter" that quantitatively predicts the depth to which particles penetrate into a given medium across diverse conditions. Our simulations also uncover a surprising cooperative effect: Adding more particles enables them to penetrate deeper into the medium. This phenomenon arises because individual particles redirect fluid to adjacent throats, forcing nearby particles through tight pores that they would otherwise clog. Altogether, these results help to establish a quantitative framework that connects microscopic particle mechanics to macroscopic transport behavior. Published by the American Physical Society 2025

Copyright and License

Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.

Acknowledgement

It is a pleasure to acknowledge Baojun Bai for useful discussions, as well as funding to S.K. through the Chateaubriand Fellowship of the Office for Science & Technology of the Embassy of France in the United States, to L.T. through the INTPART program from the Research Council of Norway (Project No. 309139), to M.R. through the Princeton Center for Complex Materials MRSEC (NSF Grant No. DMR-2011750), and to S.S.D. through NSF Grant No. DMR-2011750, the Project X Innovation Fund, the Camille Dreyfus Teacher-Scholar Program of the Camille and Henry Dreyfus Foundation (SSD). This material is also based upon work by SSD supported by the U.S. Department of Energy's Office of Energy Efficiency and Renewable Energy (EERE) under the Geothermal Technologies Office (GTO) Innovative Methods to Control Hydraulic Properties of Enhanced Geothermal Systems Award No. DE-EE0009790.

Data Availability

The data that support the findings of this article are openly available at : 

Supplemental Material

Supplemental calculations, data, and video:

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Additional details

Funding

The Research Council of Norway
309139
National Science Foundation
DMR-2011750
Materials Research Science and Engineering Centers
Camille and Henry Dreyfus Foundation
United States Department of Energy
Office of Energy Efficiency and Renewable Energy
Geothermal Technologies Office

Caltech Custom Metadata

Caltech groups
Division of Chemistry and Chemical Engineering (CCE)
Publication Status
Published