Published February 26, 2024 | Version Submitted
Discussion Paper Open

Multi-qubit gates and 'Schrödinger cat' states in an optical clock

Abstract

Many-particle entanglement is a key resource for achieving the fundamental precision limits of a quantum sensor. Optical atomic clocks, the current state-of-the-art in frequency precision, are a rapidly emerging area of focus for entanglement-enhanced metrology. Augmenting tweezer-based clocks featuring microscopic control and detection with the high-fidelity entangling gates developed for atom-array information processing offers a promising route towards leveraging highly entangled quantum states for improved optical clocks. Here we develop and employ a family of multi-qubit Rydberg gates to generate 'Schrödinger cat' states of the Greenberger-Horne-Zeilinger (GHZ) type with up to 9 optical clock qubits in a programmable atom array. In an atom-laser comparison at sufficiently short dark times, we demonstrate a fractional frequency instability below the standard quantum limit using GHZ states of up to 4 qubits. A key challenge to improving the optimal achievable clock precision with GHZ states is their reduced dynamic range. Towards overcoming this hurdle, we simultaneously prepare a cascade of varying-size GHZ states to perform unambiguous phase estimation over an extended interval. These results demonstrate key building blocks for approaching Heisenberg-limited scaling of optical atomic clock precision.

Acknowledgement

We acknowledge earlier contributions to the experiment from M. A. Norcia and N. Schine as well as fruitful discussions with R. Kaubruegger and P. Zoller. The authors also wish to thank S. Lannig and A. M. Rey for careful readings of the manuscript and helpful comments. In addition, we thankfully acknowledge helpful technical discussions and contributions to the clock laser system from A. Aeppli, M. N. Frankel, J. Hur, D. Kedar, S. Lannig, B. Lewis, M. Miklos, W. R. Milner, Y. M. Tso, W. Warfield, Z. Hu, Z. Yao. This material is based upon work supported by the Army Research Office (W911NF-19-1-0149, W911NF-19-1-0223), the Air Force Office for Scientific Research (FA9550-19-1-0275), the National Science Foundation QLCI (OMA-2016244), the U.S. Department of Energy, Office of Science, the National Quantum Information Science Research Centers, Quantum Systems Accelerator, and the National Institute of Standards and Technology. This research also received funding from the European Union’s Horizon 2020 program under the Marie Sklodowska-Curie project 955479 (MOQS), the Horizon Europe program HORIZON-CL4-2021- DIGITALEMERGING-01-30 via the project 101070144 (EuRyQa) and from the French National Research Agency under the Investments of the Future Program project ANR-21-ESRE-0032 (aQCess). We also acknowledge funding from Lockheed Martin. A.C. acknowledges support from the NSF Graduate Research Fellowship Program (Grant No. DGE2040434); W.J.E. acknowledges support from the NDSEG Fellowship; N.D.O. acknowledges support from the Alexander von Humboldt Foundation.

Contributions

A.C., W.J.E., T.L.Y., A.W.Y., N.D.O. and A.M.K. contributed to the experimental setup, performed the measurements and analyzed the data. S.J. and G.P. conceptualized the multi-qubit gate design. L.Y. and K.K. contributed to the clock laser system under supervision from J.Y. A.M.K. supervised the work. All authors contributed to the manuscript.

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arXiv.org perpetual non-exclusive license

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Additional details

Funding

United States Army Research Office
W911NF-19-1-0149
United States Army Research Office
W911NF-19-1-0223
United States Air Force Office of Scientific Research
FA9550-19-1-0275
National Science Foundation
OSI-2016244
United States Department of Energy
National Institute of Standards and Technology
European Research Council
Marie Skłodowska-Curie Fellowship 955479
European Research Council
101070144
Agence Nationale de la Recherche
ANR-21-ESRE-0032
Lockheed Martin (United States)
National Science Foundation
NSF Graduate Research Fellowship DGE-2040434
United States Department of Defense
National Defense Science and Engineering Graduate (NDSEG) Fellowship
Alexander von Humboldt Foundation