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Published January 15, 1985 | Published
Journal Article Open

Intramolecular dephasing in pyrazine: Direct picosecond time resolution


Because of its importance to the theory of radiationless transitions in isolated molecules, the problem of intramolecular dephasing and relaxation in pyrazine is perhaps the most studies case so far. In this molecule, a single state rovibronic level (JK) is coupled to a set of rovibronic triplet manifold levels, computed to be approximately 13 in number.(1)

Additional Information

© 1985 American Institute of Physics. Received 11 October 1984; accepted 2 November 1984. This work was supported by grant No. DMR-8105034 from the National Science Foundation. [A.H.Z. was a] Camille and Henry Dreyfus Foundation Teacher-Scholar. Arthur Amos Noyes Laboratory of Chemical Physics, Contribution No. 7108.

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