Published June 17, 2025 | Version Published
Journal Article Open

Prospects for measuring the electron's electric dipole moment with polyatomic molecules in an optical lattice

  • 1. ROR icon University of Groningen
  • 2. ROR icon National Institute for Subatomic Physics
  • 3. ROR icon VU Amsterdam
  • 4. ROR icon Massachusetts Institute of Technology
  • 5. ROR icon California Institute of Technology
  • 6. ROR icon National University of the Northeast
  • 7. ROR icon Comenius University

Abstract

We present the conceptual design of an experiment to measure the electron's electric dipole moment (eEDM) using ¹³BaOH molecules in an optical lattice. The BaOH molecule is laser-coolable and highly sensitive to the eEDM, making it an attractive candidate for such a precision measurement, and capturing it in an optical lattice offers potentially very long coherence times. We study possibilities and limitations of this approach, identify the most crucial limiting factors and ways to overcome them. The proposed apparatus can reach a statistical error of 10³𝑒cm by measuring spin precession on a total number of 5×10 molecules over a span of 120 days.

Copyright and License

 ©2025 American Physical Society.

Acknowledgement

We thank Yuly Chamorro, Scott Eustice, Thomas Meijknecht, Odile Smits, Michael Tarbutt, Anno Touwen, and Julian Wienand for helpful discussions.

Funding

The work of L.F.P., N.B., and S.H. is supported by Project No. VI.C.212.016 financed by the Dutch Research Council (NWO). The work of S.H., A.B., T.F., and I.A.A. is supported by the ENW-M2 NWO Grant No. OCENW.M.21.098. The work of S.H., A.B., and E.P. is supported by ENW-XL NWO Grant No. OCENW.XL21.XL21.074. I.A.A. acknowledges partial support from FONCYT through Grants No. PICT-2021-I-A-0933 and No. PICT-2020-SerieA-0052, and from CONICET through Grant No. PIBAA-2022-0125CO.

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Additional details

Related works

Is new version of
Discussion Paper: arXiv:2411.00441 (arXiv)

Funding

Dutch Research Council
VI.C.212.016
Dutch Research Council
OCENW.M.21.098
Dutch Research Council
OCENW.XL21.XL21.074
Agencia Nacional de Promoción de la Investigación, el Desarrollo Tecnológico y la Innovación
PICT-2021-I-A-0933
Agencia Nacional de Promoción de la Investigación, el Desarrollo Tecnológico y la Innovación
PICT-2020-SerieA-0052
Consejo Nacional de Investigaciones Científicas y Técnicas
PIBAA-2022-0125CO

Dates

Accepted
2025-06-03

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Caltech groups
Division of Physics, Mathematics and Astronomy (PMA)
Publication Status
Published