Hyperbolic phonon-polariton electroluminescence in 2D heterostructures
Abstract
Phonon polaritons are quasiparticles resulting from the coherent coupling of photons with optical phonons in polar dielectrics1. Owing to their exceptional ability to confine electric fields to deep-subwavelength scales with low loss, they are uniquely poised to enable a suite of applications beyond the reach of conventional photonics, such as subdiffraction imaging and near-field energy transfer. The conventional approach to exciting phonon polaritons through optical methods, however, involves costly light sources along with near-field schemes, and generally leads to low excitation efficiency owing to substantial momentum mismatch between phonon polaritons and free-space photons. Here we demonstrate that under proper conditions, phonon polaritons can be excited all-electrically by drifting charge carriers. Specifically, in hexagonal boron nitride (hBN)/graphene heterostructures, by electrically driving charge carriers in ultrahigh-mobility graphene out of equilibrium, we observe bright electroluminescence of hBN's hyperbolic phonon polaritons (HPhPs) at mid-infrared frequencies, which shows a temperature and carrier density dependence distinct from black-body thermal emission. Moreover, the carrier density dependence of the HPhP electroluminescence spectra reveals that HPhP electroluminescence can arise from both interband transition and intraband Cherenkov radiation of charge carriers in graphene. The HPhP electroluminescence offers avenues for realizing electrically pumped mid-infrared and terahertz phonon-polariton light sources.
Copyright and License
© The Author(s), under exclusive licence to Springer Nature Limited 2025.
Acknowledgement
We thank R. Yu, M. He, J. Garcia de Abajo, J. Khurgin and F. Guinea for discussions. Q.G. and G.H. acknowledge the support from the Advanced Science Research Center and the Graduate Center of the City University of New York through the start-up grant. Research at Yale University was supported by the National Science Foundation CAREER Award (ECCS-1552461) and Yale University through the start-up grant. E.D. acknowledges support from the SNSF project 200021-212899 and the ARO grant number W911NF-21-1-0184. J.H.E. acknowledges the support of the Materials Engineering and Processing programme of the National Science Foundation, award number CMMI 1538127. G.R. expresses gratitude for the support by the Simons Foundation, and the ARO MURI grant number W911NF-16-1-0361. I.E. is grateful for support from the Simons Foundation and the Institute of Quantum Information and Matter.
Contributions
These authors contributed equally: Qiushi Guo, Iliya Esin, Cheng Li.
Q.G. and F.X. conceived the idea. Q.G. and C.L. fabricated the devices and performed the measurements with assistance from C.C. I.E. performed the theoretical modelling and physical interpretation of the carrier transport and the HPhP electroluminescence, with inputs from G.R. and E.D. S.L. and J.H.E. synthesized the h10BN. Q.G. performed the optical simulation with assistance from G.H. and S.Z. Q.G. and I.E. wrote the paper with inputs from all authors. E.D., G.R. and F.X. supervised the project.
Data Availability
The data used to produce the plots in this work are available at https://doi.org/10.6084/m9.figshare.25237654.
Code Availability
The code for our theoretical model is available at https://doi.org/10.6084/m9.figshare.25237654.
Supplemental Material
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Additional details
- City University of New York
- National Science Foundation
- ECCS-1552461
- Yale University
- Swiss National Science Foundation
- 200021-212899
- United States Army Research Office
- W911NF-21-1-0184
- National Science Foundation
- CMMI-1538127
- Simons Foundation
- United States Army Research Office
- W911NF-16-1-0361
- Accepted
-
2025-01-22
- Available
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2025-03-19Published
- Caltech groups
- Institute for Quantum Information and Matter, Division of Engineering and Applied Science (EAS), Division of Physics, Mathematics and Astronomy (PMA)
- Publication Status
- Published