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Published December 1, 2023 | Published
Journal Article Open

The Wiedemann-Franz law in doped Mott insulators without quasiparticles

Abstract

Many metallic quantum materials display anomalous transport phenomena that defy a Fermi liquid description. Here, we use numerical methods to calculate thermal and charge transport in the doped Hubbard model and observe a crossover separating high- and low-temperature behaviors. Distinct from the behavior at high temperatures, the Lorenz number L becomes weakly doping dependent and less sensitive to parameters at low temperatures. At the lowest numerically accessible temperatures, L roughly approaches the Wiedemann-Franz constant L₀, even in a doped Mott insulator that lacks well-defined quasiparticles. Decomposing the energy current operator indicates a compensation between kinetic and potential contributions, which may help to clarify the interpretation of transport experiments beyond Boltzmann theory in strongly correlated metals.

Copyright and License

© 2023 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. This is an article distributed under the terms of the Science Journals Default License.

Acknowledgement

We acknowledge helpful discussions with A. Auerbach, D. Belitz, E. Berg, S. A. Hartnoll, N. E. Hussey, S. A. Kivelson, P. A. Lee, R. T. Scalettar, Z. X. Shen, and E. Tulipman.

Funding

This work was supported by the US Department of Energy (DOE), Office of Basic Energy Sciences, Division of Materials Sciences and Engineering. E.W.H. was supported by the Gordon and Betty Moore Foundation EPiQS Initiative through the grants GBMF 4305 and GBMF 8691. Y.S. was supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through grants GBMF 4302 and GBMF 8686. Y.S.'s contribution to the work was done prior to joining AWS Center for Quantum Computing. Computational work was performed on the Sherlock cluster at Stanford University and on resources of the National Energy Research Scientific Computing Center, supported by the US DOE, Office of Science, under Contract no. DE-AC02-05CH11231.

Contributions

W.O.W. and T.P.D. conceived the study. W.O.W. performed numerical simulations and conducted data analysis and interpretation. J.K.D., Y.S., E.W.H., B.M., and T.P.D. assisted in data interpretation. W.O.W., B.M., and T.P.D. wrote the manuscript with input from all coauthors.

Data Availability

Code and data presented in this study are deposited in Zenodo (41, 42).

Conflict of Interest

The authors declare no competing interests.

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Additional details

Created:
December 1, 2023
Modified:
December 1, 2023