Published July 4, 2025 | Version Published
Journal Article Open

Efficient and wavelength-tunable second-harmonic generation toward the green gap

  • 1. ROR icon California Institute of Technology
  • 2. ROR icon University of California, Santa Barbara

Abstract

Achieving compact and efficient visible laser sources is crucial for a wide range of applications. However, traditional semiconductor laser technology faces difficulties in producing high-brightness green light, leaving a “green gap” in wavelength coverage. Second-harmonic generation (SHG) offers a promising alternative by converting near-infrared sources to visible wavelengths with high efficiency and spectral purity. Here, we demonstrate efficient and tunable SHG within the green spectrum using a high-Q Si3N4 microresonator. On-chip green power as high as 5.3 milliwatts is generated with a conversion efficiency of 141% per watt (absolute 7.9%). A space-charge grating induced by the photogalvanic effect realizes reconfigurable grating numbers and flexible wavelength tuning over a range of 2.6 terahertz. In addition, grating formation dynamics and competition are observed. These findings underscore the potential of Si3N4 as a robust, integrative platform for on-chip, tunable green light sources.

Copyright and License

© 2025 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution License 4.0 (CC BY).

Funding

This work was supported by the Defense Advanced Research Projects Agency (HR001-20-2-0044), the Air Force Office of Scientific Research (FA9550-23-1-0587), and the Kavli Nanoscience Institute at Caltech.

Data Availability

All data needed to evaluate the conclusions in the paper are present in the paper. The data that support the plots within this paper and other findings of this study are available at Dryad (https://datadryad.org/share/2m5i38SSzasdEWbZii1B0yq86Y89d6NdMPe2zmkgbU8).

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Additional details

Identifiers

Related works

Has version
Journal Article: PMC12219504 (PMCID)
Is new version of
Discussion Paper: arXiv:2504.17869 (arXiv)
Is supplemented by
Dataset: https://datadryad.org/share/2m5i38SSzasdEWbZii1B0yq86Y89d6NdMPe2zmkgbU8 (URL)

Funding

Defense Advanced Research Projects Agency
HR001-20-2-0044
United States Air Force Office of Scientific Research
FA9550-23-1-0587
California Institute of Technology
Kavli Nanoscience Institute -

Dates

Accepted
2025-05-27
Available
2025-07-02
Published

Caltech Custom Metadata

Caltech groups
Kavli Nanoscience Institute, Division of Engineering and Applied Science (EAS)
Publication Status
Published