Published November 15, 1969 | Version public
Journal Article

The proper treatment of off-diagonal Lagrange multipliers and coupling operators in self-consistent field equations

  • 1. ROR icon Jet Propulsion Lab

Abstract

We show that past treatments of the off-diagonal Lagrange multipliers or coupling operators in the self-consistent field equations for open-shell systems and in the multi-configuration SCF equations are incomplete. In addition, we obtain the complete variational equations and show how these may be combined into one simple eigenvalue problem which is solved for all orbitals.

Additional Information

© 1969 Published by Elsevier B.V. Received 12 September 1969. Partially supported by grants (GP-6965) and (GP-15423) from the National Science Foundation. Arthur Amos Noyes Laboratory of Chemical Physics Contribution No. 3940

Additional details

Identifiers

Eprint ID
87804
DOI
10.1016/0009-2614(69)80170-3
Resolver ID
CaltechAUTHORS:20180712-121222509

Related works

Funding

NSF
GP-6965
NSF
GP-15423
Alfred P. Sloan Foundation
NSF Predoctoral Fellowship
NDEA Fellowship

Dates

Created
2018-07-12
Created from EPrint's datestamp field
Updated
2021-11-15
Created from EPrint's last_modified field

Caltech Custom Metadata

Other Numbering System Name
Arthur Amos Noyes Laboratory of Chemical Physics
Other Numbering System Identifier
3940