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Published June 1, 2024 | v1
Journal Article

A perspective of recent advances in PECVD-grown graphene thin films for scientific research and technological applications

  • 1. ROR icon California Institute of Technology

Abstract

The purpose of this review is to provide a perspective on some of the recent advances in applying graphene thin films, including monolayer and multilayer graphene sheets synthesized by a scalable approach based on plasma-enhanced chemical vapor deposition (PECVD), to scientific research and technologies. The technological applications present here include the use of graphene in flexible electronics, for anticorrosion of metals, and for Si-based technologies including superlubricity and optoelectronics. In the case of fundamental scientific research, we demonstrate that periodic patterns of nanoscale strain distributions in monolayer graphene can lead to local giant pseudomagnetic fields as well as global modifications to the electronic properties of monolayer graphene, including strain-induced valley Hall signals and quantized Landau levels in the absence of external magnetic fields, edge states, as well as increasing electronic correlation with increasing strain. These findings suggest new approaches towards developing emerging quantum states with tunable electronic correlation based on graphene straintronics.

    Copyright and License

    © 2024 Elsevier.

    Acknowledgement

    The research presented in this review was jointly supported by the Industrial Technology Research Institute (ITRI) in Taiwan (NCY.PECVD3-1-ITRI.SRA2022), the National Science Foundation under the Physics Frontier Centers program for the Institute for Quantum Information and Matter (IQIM) at Caltech (Award #1733907), and the Army Research Office under the MURI program (award #W911NF-16-1-0472). C.-H. Lu acknowledges a fellowship from the J. Yang & Family Foundation. D. Hao acknowledges partial support from the Eddleman graduate fellowship program under IQIM at Caltech. N.-C. Yeh acknowledges partial support from the Thomas W. Hogan Professorship at Caltech, the Yushan Fellowship awarded by the Ministry of Education in Taiwan, and the Yushan Fellow Distinguished Professorship at the National Taiwan Normal University in Taiwan. The authors are grateful to Professor Patrick A. Lee for stimulus discussions on the physics of graphene straintronics.

    Data Availability

    Data will be made available on request.

    Conflict of Interest

    The authors declare the following financial interests/personal relationships which may be considered as potential competing interests:

    Nai-Chang Yeh reports financial support was provided by California Institute of Technology. Nai-Chang Yeh reports financial support was provided by National Science Foundation. Nai-Chang Yeh reports financial support was provided by US Army Research Laboratory. Chen-Hsuan Lu reports financial support was provided by Industrial Technology Research Institute, Taiwan. Duxing Hao reports financial support was provided by National Science Foundation. Duxing Hao reports financial support was provided by US Army Research Laboratory. Nai-Chang Yeh reports financial support was provided by Ministry of Education, Taiwan.

    Additional Information

    This article is a part of the Virtual Special Issue on Carbon Films. This issue is in memory of Professor Mildred S. Dresselhaus of Massachusetts Institute of Technology. The editor of this issue is Professor D.D.L. Chung of University at Buffalo, The State University of New York.

    Additional details

    Created:
    May 30, 2024
    Modified:
    May 30, 2024