Single-pulse ultrafast real-time simultaneous planar imaging of femtosecond laser-nanoparticle dynamics in flames
Abstract
The creation of carbonaceous nanoparticles and their dynamics in hydrocarbon flames are still debated in environmental, combustion, and material sciences. In this study, we introduce single-pulse femtosecond laser sheet-compressed ultrafast photography (fsLS-CUP), an ultrafast imaging technique specifically designed to shed light on and capture ultrafast dynamics stemming from interactions between femtosecond lasers and nanoparticles in flames in a single-shot. fsLS-CUP enables the first-time real-time billion frames-per-second (Gfps) simultaneous two-dimensional (2D) imaging of laser-induced fluorescence (LIF) and laser-induced heating (LIH) that are originated from polycyclic aromatic hydrocarbons (PAHs) and soot particles, respectively. Furthermore, fsLS-CUP provides the real-time spatiotemporal map of femtosecond laser-soot interaction as elastic light scattering (ELS) at an astonishing 250 Gfps. In contrast to existing single-shot ultrafast imaging approaches, which are limited to millions of frames per second only and require multiple laser pulses, our method employs only a single pulse and captures the entire dynamics of laser-induced signals at hundreds of Gfps. Using a single pulse does not change the optical properties of nanoparticles for a following pulse, thus allowing reliable spatiotemporal mapping. Moreover, we found that particle inception and growth are derived from precursors. In essence, as an imaging modality, fsLS-CUP offers ultrafast 2D diagnostics, contributing to the fundamental understanding of nanoparticle’s inception and broader applications across different fields, such as material science and biomedical engineering.
Copyright and License
Open Access. This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made.
Acknowledgement
Y.N.M. gratefully acknowledges the Swedish Research Council for the financial support of grant # IPD2018-06783. Part of the work of Y.N.M. that was enabled by JPL was carried out at the Jet Propulsion Laboratory, California Institute of Technology, under a contract with NASA (80NM0018D0004). MSG thanks funding from JPL JROC and NASA SSW programs.
Conflict of Interest
The authors disclose the following patents for the CUP technology: WO2016085571 A3 (L.V.W.) and US10992924B2 (L.V.W. and P.W.).
Supplemental Material
Code Availability
The reconstruction algorithm is described in detail in Supplementary Information. We have opted not to make the computer code publicly available because the code is proprietary and used for other projects.
Supplementary information accompanies the manuscript on the Light: Science & Applications website (http://www.nature.com/lsa).
Contributions
Y.N.M. proposed the fsLS-CUP of soot and PAHs. P.W. and Y.N.M. designed, built and characterized the fsLS-CUP system. P.W. and Y.N.M. performed the experiments. P.W. and Y.N.M. developed the image processing algorithm and conducted the image reconstruction. F.J.B. performed numerical modeling. Y.N.M., P.W., and F.J.B. analyzed the experimental data and drafted the manuscript. M.S.G. reviewed the technical details and advised on evaluation approaches. L.V.W. supervised the project. All authors revised the manuscript.
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Additional details
- Swedish Research Council
- IPD2018-06783
- Accepted
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2024-08-15Accepted
- Available
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2024-08-29Published online
- Publication Status
- Published