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Published August 15, 1985 | Published
Journal Article Open

Picosecond monitoring of a chemical reaction in molecular beams: Photofragmentation of R–I→R‡+I


Studies of chemical reactions by molecular beam techniques and spectroscopic methods have provided extensive information on the nature of the intermediates involved and on the energy distribution in products.(1-6) Until now, however, there is no report of direct picoseconds time resolution of a chemical reaction in molecular beams.

Additional Information

© 1985 American Institute of Physics. Received 15 May 1985; accepted 11 June 1985. This research was supported by a grant from the National Science Foundation. We thank Professor R. Marcus, Professor R. Bernstein, Professor W. Goddard, and Professor J. Beauchamp for enlightening discussions. This work was presented at the International Conference "Recent Advances in Molecular Reaction Dynamics," Aussois, France, June 1985. [A.H.Z. was a] Camille and Henry Dreyfus Teacher-Scholar. Arthur Amos Noyes Laboratory of Chemical Physics, Contribution No. 7189.

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